Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine

International journal of scientific report, 23 p.

-д хадгалсан:
Номзүйн дэлгэрэнгүй
Үндсэн зохиолчид: Mphuthi, Ntsoaki, Adekunle, Abolanle S., Fayemi, Omolola E., Olasunkanmi, Lukman O., Ebenso, Eno E.
Формат: Сэтгүүл
Хэл сонгох:англи
Хэвлэсэн: Springer publishing 2020
Нөхцлүүд:
Онлайн хандалт:https://ir.oauife.edu.ng/handle/123456789/5113
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author Mphuthi, Ntsoaki
Adekunle, Abolanle S.
Fayemi, Omolola E.
Olasunkanmi, Lukman O.
Ebenso, Eno E.
author_facet Mphuthi, Ntsoaki
Adekunle, Abolanle S.
Fayemi, Omolola E.
Olasunkanmi, Lukman O.
Ebenso, Eno E.
author_sort Mphuthi, Ntsoaki
collection DSpace
description International journal of scientific report, 23 p.
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id oai:ir.oauife.edu.ng:123456789-5113
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language English
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spelling oai:ir.oauife.edu.ng:123456789-51132023-05-13T11:10:23Z Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine Mphuthi, Ntsoaki Adekunle, Abolanle S. Fayemi, Omolola E. Olasunkanmi, Lukman O. Ebenso, Eno E. Phthalocyanine Metal Oxide electrocatalytic nanoparticles Electrocatalytic oxidation International journal of scientific report, 23 p. The electrocatalytic properties of metal oxides (MO=Fe3O4, ZnO) nanoparticles doped phthalocyanine (Pc) and functionalized MWCNTs, decorated on glassy carbon electrode (GCE) was investigated. Successful synthesis of the metal oxide nanoparticles and the MO/Pc/MWCNT composite were confirmed using UV-Vis, EDX, XRD and TEM techniques. Successful modification of GCE with the MO and their composite was also confirmed using cyclic voltammetry (CV) technique. GCE-MWCNT/ ZnO/29H,31H-Pc was the best electrode towards DA detection with very low detection limit (0.75μM) which compared favourably with literature, good sensitivity (1.45μA/μM), resistance to electrode fouling, and excellent ability to detect DA without interference from AA signal. Electrocatalytic oxidation of DA on GCE-MWCNT/ZnO/29H,31H-Pc electrode was diffusion controlled but characterized with some adsorption of electro-oxidation reaction intermediates products. The fabricated sensors are easy to prepare, cost effective and can be applied for real sample analysis of dopamine in drug composition. The good electrocatalytic properties of 29H,31H-Pc and 2,3-Nc were related to their (quantum chemically derived) frontier molecular orbital energies and global electronegativities. The better performance of 29H,31H-Pc than 2,3-Nc in aiding electrochemical oxidation of DA might be due to its better electron accepting ability, which is inferred from its lower ELUMO and higher χ. 2020-01-21T11:48:58Z 2020-01-21T11:48:58Z 2017-03-03 Journal Mphuthi, Ntsoaki & Adekunle, Abolanle & Fayemi, Omolola & Olasunkanmi, Lukman & Ebenso, Eno. (2017). Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine. Scientific Reports. 7. 43181. 10.1038/srep43181. DOI: 10.1038/srep43181 https://ir.oauife.edu.ng/handle/123456789/5113 en application/pdf Springer publishing
spellingShingle Phthalocyanine
Metal Oxide
electrocatalytic
nanoparticles
Electrocatalytic oxidation
Mphuthi, Ntsoaki
Adekunle, Abolanle S.
Fayemi, Omolola E.
Olasunkanmi, Lukman O.
Ebenso, Eno E.
Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine
title Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine
title_full Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine
title_fullStr Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine
title_full_unstemmed Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine
title_short Phthalocyanine Doped Metal Oxide Nanoparticles on Multiwalled Carbon Nanotubes Platform for the detection of Dopamine
title_sort phthalocyanine doped metal oxide nanoparticles on multiwalled carbon nanotubes platform for the detection of dopamine
topic Phthalocyanine
Metal Oxide
electrocatalytic
nanoparticles
Electrocatalytic oxidation
url https://ir.oauife.edu.ng/handle/123456789/5113
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